Sculpts SD Volks Girl Sculpts

Volks Super Dollfie "GOSICK" Victorique de Blois | #457176811
Victorique from Gosick was a Super Dollfie that might meet your requirements

 

Maybe SD Mika, I looove her big eyes

 

She might be hard to find, but Suiseiseki / Souseiseki (they’re the same sculpt) has huge eyes

 

I think the Volks girl with the biggest eyes is probably Nono. ❤️

 

I may be biased, but I believe my baby girl Jill- Volks saki 59 is just beautiful

 

Nayu, Nao and Mimi also have huge eyes!
Neo Angel Den lists most FCS sculpts with pictures and gives a great overview of what's there.

 

I think F22 / Kun has lovely big eyes and a hint of a smile. Sweet & mysterious.